Win Forms RadioButton controls are designed to give users a choice among two or more settings, of which only one can be assigned to a procedure or object. For example, a group of RadioButton controls may display a choice of package carriers for an order, but only one of the carriers will be used. Therefore only one RadioButton at a time can be selected, even if it's a part of a functional group.
You group radio buttons by drawing them inside a container such as a Panel control, a GroupBox control, or a form. All radio buttons that are added directly to a form become one group. To add additional groups, you need to place them inside panels or group boxes. For more information on panels or group boxes, see Panel Control and GroupBox Control.
To group RadioButton controls to function as a set
RadioButton Control | Panel Control| GroupBox Control | CheckBox Control